Laser radiation sources with wide wavelength tunability are of high demand in many applications including nonlinear microscopy, material science, spectroscopy, gas sensing, etc. Laser wavelength tunability is usually very limited, so optical parametric amplifiers (OPA) and optical parametric generators (OPGs) are used as sources of tunable laser radiation. Rapid progress in nonlinear optics enabled creation of a wide range of optical parametric devices with wavelength tunability from VIS to mid-IR spectrum range using pump from CW radiation to femtosecond pulses. However, there are very few optical parametric devices that operate in the subnanosecond duration range are (300 ps - 1 ns) and the few that have been demonstrated operate mainly in the IR spectral range. Since there is a demand of such sources in applications like laser-induced fluorescence, detection of chemical materials, etc., developing subnanosecond optical parametric devices remains an important task.
In this study we report, to the best of our knowledge, the first subnanosecond OPAs systems generating widely-tunable radiation in the visible spectrum range. The first demonstrated OPA is based on LBO crystal and the other one - on BBO crystal. To overcome difficulties related to low pump intensity and laser induced damage threshold (LIDT) of nonlinear crystals, we use continuum generated in a photonic crystal fiber as a seed source for the OPAs. Experimental data and numerical simulation reveal that good spectral, temporal and particularly energy characteristics of the seed radiation are crucial in order to achieve efficient parametric generation of signal radiation.
This work has received funding from European Regional Development Fund (project No. 01.2.2-LMT-K-718-03-0004) under grant agreement with the Research Council of Lithuania (LMTLT).
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