Here, we demonstrated vivid structural coloration and polarization-sensitive color metasurfaces using bandgap-engineered a-Si:H, whose extinction coefficient is near zero at the entire visible spectrum. The scattering response of high-index nanostructures is numerically analyzed with multipole expansion, and we vitrify that the low-optical losses of bandgap-engineered a-Si:H significantly improve color coverage of metasurface, achieving comparable coverage with the Adobe RGB gamut. Also, we demonstrated the application of optical encryption with polarization-sensitive structural coloration, achieving near-zero reflection when optical information is encrypted. We believe that structural coloration with low-loss a-Si:H will be widely used with its advantageous benefits compared to chemical pigments.
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