To enhance the PETawatt Aquitaine Laser (PETAL) operation, efforts are directed towards increasing the Laser-Induced Damage Threshold (LIDT) of transport mirrors. Three approaches are being considered : i) changing the design of thin film stacks, ii) the materials, and iii) the deposition process.
Monolayers of pure SiO2, HfO2, Sc2O3 and mixtures of HfO2/SiO2 and Sc2O3/SiO2 were elaborated by magnetron sputtering using oxide targets. Laser damage tests, combined with optical and physicochemical characterizations, revealed that the Sc2O3/SiO2 mixture exhibits the highest LIDT. The introduction of a small amount of oxygen into the plasma reduced the refractive index and improved the LIDT.
A Bragg mirror, designed for PETAL's specifications (R > 99% at 1053 nm for s polarization at 45° incidence) is being manufactured using HfO2 (high refractive index) and Sc2O3/SiO2 (low refractive index). The films thicknesses are finely controlled with the quartz crystal microbalance technique.
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