Vladimir M. Shalaev,1 Colton Fruhling,1 Sarah N. Chowdhury,1 Kang Wang,1 Wenhao Shao,1 Ludamila Prokopeva,1 Benjamin T. Diroll,2 Richard Schaller,2 Letian Dou,1 Alexander V. Kildishevhttps://orcid.org/0000-0002-8382-8422,1 Alexandra Boltasseva1
1Purdue Univ. (United States) 2Argonne National Lab. (United States)
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Quasi-2D perovskites have gained significant attention in the field of optics and photonics recently due to their intriguing optical properties. Endowed with optical properties typically found in both 2D and 3D systems, they offer a premier platform for tunable optical devices. Here we studied the prospects of Quasi-2D perovskites for lasing by first delving into excitonic and free carrier ultrafast dynamics, exploring into random lasing from naturally formed cavities in planar films and investigating lasing from structurally-tuned nanowires. Our results give insights on the fundamental radiative processes in these novel materials and build a foundation for future experiments and applications.
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Vladimir M. Shalaev, Colton Fruhling, Sarah N. Chowdhury, Kang Wang, Wenhao Shao, Ludamila Prokopeva, Benjamin T. Diroll, Richard Schaller, Letian Dou, Alexander V. Kildishev, Alexandra Boltasseva, "Lasing dynamics in dimensionality controlled quasi-2d perovskites," Proc. SPIE PC13109, Metamaterials, Metadevices, and Metasystems 2024, PC1310902 (3 October 2024); https://doi.org/10.1117/12.3027486