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3 October 2024 A tunable nanocube-on-mirror Fabry-Pérot cavity for sideband-resolved molecular optomechanics
Femius Koenderink, Ilan Shlesinger, Ewold Verhagen
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Proceedings Volume PC13110, Active Photonic Platforms (APP) 2024; PC131100H (2024) https://doi.org/10.1117/12.3027473
Event: Nanoscience + Engineering, 2024, San Diego, California, United States
Abstract
We demonstrate a tuneable nanocube-on-mirror Fabry-Perot cavity that combines the record breaking plasmonic confinement of the nanocube-on-mirror (NCoM) system with the high quality factors and tuneability of microcavity systems. We demonstrate selective addressing of individual molecular vibrational lines with robust SERS enhancements on par with those of the seminal NCoM system, reaching sideband resolved SERS at Q/V values above 1 million inverse cubic wavelengths. We envision this as a platform for sideband-resolved molecular optomechanics, polariton chemistry and vibrational strong coupling.
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Femius Koenderink, Ilan Shlesinger, and Ewold Verhagen "A tunable nanocube-on-mirror Fabry-Pérot cavity for sideband-resolved molecular optomechanics", Proc. SPIE PC13110, Active Photonic Platforms (APP) 2024, PC131100H (3 October 2024); https://doi.org/10.1117/12.3027473
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KEYWORDS
Optomechanical design
Plasmonics
Antennas
Molecules
Raman scattering
Vibration
Optical microcavities
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