Transmittance-control devices, such as a suspended particle device, electrochromic device, and dye-doped liquid crystal (LC) device, have been studied for a smart window, eyewear, and automotive applications. These devices require a high transmittance difference between the transparent and opaque states. Among the dye-doped LC devices, a dye-doped chiral-nematic LC (CNLC) cell has been widely used for transmittance-control devices. However, the colors of cells are different between the homogeneously aligned and CNLC cell. In this study, we demonstrated a systematic approach to find optimum dye concentrations for black color in a dye-doped CNLC cell. We took its transmission spectrum into account in the numerical calculation to realize the black color in a dye-doped CNLC cell. Through the iterative method, we could optimize the concentration of each single dye for realizing the black color. We confirmed that a dye-doped CNLC cell designed by considering transmission spectrum of it could provide the black color in the CIE 1931 color space.
Light shutter technologies that can control optical transparency have been studied extensively for developing curtain-free smart windows. We introduce thermally and optically switchable light shutters using LCs doped with push-pull azobenzene, which is known to speed up thermal relaxation. The liquid crystal light shutter can be switched between translucent and transparent states or transparent and opaque states by phase transition through changing temperature or photo-isomerization of doped azobenzene. The liquid crystal light shutter can be used for privacy windows with an initial translucent state or energy-saving windows with an initial transparent state.
We propose a smart window using polymer-networked liquid crystals doped with push-pull azobenzene. Azobenzene is used to provide phase transition from the nematic to isotropic state through the trans-cis isomerization of azobenzene. When exposed to sunlight, the device switches from the opaque nematic phase to the transparent isotropic phase. Switching from the transparent to opaque state can be obtained through rapid cis-trans isomerization of push-pull azobenzene without sunlight exposure. The proposed device can reduce the transmittance of the incident sunlight during daytime, whereas it can scatter the incident light during the night for privacy.
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