Weyl semimetals are a group of materials with a single touching point of valence and conduction bands and a linear electron dispersion in the adjacent electronic bandstructure, giving rise quasi-massless electrons and topologically protected surface states. However, previous works on Weyl semimetals were largely limited to bulk material and therefore limited in means of flexibility and on-chip device applications.
Our work demonstrates first steps towards nanophotonics applications with Weyl semimetals by thoroughly characterizing the linear and nonlinear optical properties of recently realized epitaxial grown thin films of the prototypical Weyl semimetal niobium phosphide (NbP). Despite the dominant absorption over the entire spectrum, pronounced third-harmonic generation could be detected, reaching a maximum efficiency of 10-4 %, being orders of magnitude higher than for common dielectric materials. Furthermore, non-degenerate pump-probe measurements with 10 fs pulses were performed to investigate the ultrafast electronic and optical response of bulk NbP crystal and NbP thin film. For the first, absorption effects and subsequent scattering processes dominate the ultrafast response and show the characteristics of the linear dispersion regime in the electronic bandstructure. On the other hand, the NbP thin films reveal a response that is generated by the nonlinear optical Kerr effect and gives an ultrafast modulation depth of close to 1 % and with a complete relaxation within 100 fs. These findings would allow all-optical switching based on NbP with full-width half maximum bandwidth of 10-20 MHz.
Altogether, our results show that the epitaxial grown NbP thin films inherit the optical properties of the bulk crystal and further boost the nonlinear optical interactions. Combined with the possibility of common top-down fabrication techniques enabled by thin films, this paves the way for future applications of nanophotonic devices based on the promising properties of Weyl semimetals.
Non-collinear magnets (NCM) exhibit a spatial variation of the magnetization direction, where helical and skyrmionic spin orders in materials have lately attracted considerable interest. This interest is spurred by both, exploring the physical origin of nanoscale NCM and applications in spintronics. Our study advances the understanding of nanoscale NCM by revealing the effect of nanoscale lateral confinement on the physical properties of NCM.
We combine spin-polarized scanning tunneling microscopy/spectroscopy (sp-STM/S) and first-principles calculations to study prototypical helical NCM of some nm extension in proximity to both ferromagnetic Co and vacuum regions. We report a non-uniform distortion of the spin helix in an Fe bilayer on Cu(111)[1], where the spin orientation deviates from that of an ideal helical structure. The proximity to either Co or vacuum leads to distortions of the spin orientation within nm range of the respective interface. The distortions give rise to a specific energy dependent phenomenon of non-collinearity between the local magnetization in the sample and the electronic magnetization probed above its surface. This phenomenon is a direct consequence of the spinor nature of the electronic states in NCM. The symmetry breaking due to lateral confinement makes the spinor nature of electronic states observable in sp-STM/S experiments.
[1] Phark, S. H.; Fischer, J. A.; Corbetta, M.; Sander, D.; Nakamura, K. and Kirschner, J. Reduced-dimensionality-induced helimagnetism in iron nanoislands Nat. Commun. 5 (2014) 5183.
David Carlton, Brian Lambson, Zheng Gu, Scott Dhuey, Li Gao, Brian Hughes, Deirdre Olynick, Charles Rettner, Andreas Scholl, Brian Youngblood, Anthony Young, Ilya Krivorotov, Stuart Parkin, Jeffrey Bokor
As conventional Silicon-based transistors reach their scaling limits, novel devices for performing computations have
emerged as alternatives to continue the improvements in information technology that have benefited society over the
past 40 years. One candidate that has shown great promise recently is a device that performs logical computations using
dipole coupled nanomagnets. In this paper, we discuss recent advances that have led to a greater understanding of signal
propagation in nanomagnet arrays. In particular, we highlight recent experimental work towards the imaging of a
propagating magnetic cascade.
Multilayer films such as (Co/Pt) are considered to be potential candidates for future high density optical recording media, since they exhibit a strong magneto-optic Kerr activity at wavelengths less than about 500 nm. The magnetic properties of those multilayer films, however, are very sensitive to the way the films are grown, and thus it is the key for achieving better performance to understand how they are correlated to the microstructure. Very little understanding has ever been achieved as to the correlation between the microstructure and the magnetic properties. This is particularly so for the coercivity, which is the important factor governing the domain shape and its size. In view of this aspect, we have systematically examined how the fabrication condition affects the microstructure of both Co/Pt and Fe/Pt multilayer films and in turn influences the magnetic properties.
Conference Committee Involvement (1)
Oxide-based Materials and Devices
24 January 2010 | San Francisco, California, United States
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