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Spectra of the Raman scattering (RS) by transverse and longitudinal A1-vibrations in crystals of the lithium niobate and lithium tantalate are investigated at room and liquid helium temperatures. An essential decrease of the RS- linewidths for scattering by A1T-phonons is found in the course of deceasing from room to liquid helium temperature. The obtained results show that coherent excitation of polariton modes in ferroelectrics is a promising method for generating the frequency-tunable submillimeter-band radiation.
Vladimir S. Gorelik,Alexandr L. Karuzskii,Anatolii V. Perestoronin, andPavel P. Sverbil
"Raman scattering by phonons and polaritons in LiNbO3 and LiTaO3", Proc. SPIE 4069, Raman Scattering, (18 February 2000); https://doi.org/10.1117/12.378136
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Vladimir S. Gorelik, Alexandr L. Karuzskii, Anatolii V. Perestoronin, Pavel P. Sverbil, "Raman scattering by phonons and polaritons in LiNbO3 and LiTaO3," Proc. SPIE 4069, Raman Scattering, (18 February 2000); https://doi.org/10.1117/12.378136