Stimulated Raman scattering in new organic and inorganic crystalline materials

Hanjo Rhee; Alexander A. Kaminskii; Hans Joachim Eichler

doi:10.1117/12.701329

14 February 2007 Stimulated Raman scattering in new organic and inorganic crystalline materials

Hanjo Rhee, Alexander A. Kaminskii, Hans Joachim Eichler

Proceedings Volume 6455, Nonlinear Frequency Generation and Conversion: Materials, Devices, and Applications VI; 64550T (2007) https://doi.org/10.1117/12.701329
Event: Lasers and Applications in Science and Engineering, 2007, San Jose, California, United States

Abstract

Results of our SRS investigations of the organic crystals &agr;-Ca(HCOO)₂ (alpha calcium formate), LiNH₂C₆H₄SO₃ • H₂O (lithium sulfanilate monohydrate) and N(CH₂CH₂NH₃)₃Br₃ (tren trihydrobromide) are presented. Currently a promising development in solid-state laser physics is the use of highly transparent ceramics. We have demonstrated efficient SRS in three ceramics based on cubic rare earth sesquioxides RE₂O₃ (RE = Sc, Y and Lu) with Raman shifts in the range of 378 cm^-1 to 419 cm^-1. Cascading &khgr;⁽³⁾ → &khgr;⁽²⁾ → &khgr;⁽³⁾ lasing effects, self-SHG, self-SFM and cascading Stokes and anti-Stokes generation between phonons of different energies has been observed in Li₂SO₄ • H₂O (lithium sulphate monohydrate), CsLiMoO₄ (caesium lithium molybdate) and CsLiMoO₄ • 1/3H₂O.

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Hanjo Rhee, Alexander A. Kaminskii, and Hans Joachim Eichler "Stimulated Raman scattering in new organic and inorganic crystalline materials", Proc. SPIE 6455, Nonlinear Frequency Generation and Conversion: Materials, Devices, and Applications VI, 64550T (14 February 2007); https://doi.org/10.1117/12.701329

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KEYWORDS

Raman spectroscopy

Crystals

Ceramics

Nonlinear crystals

Second-harmonic generation

Lithium

Phonons

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