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Highly ordered iron incorporated mesoporous silica (Fe-SBA15) was prepared and used as a template for catalytic
polymerization of functional molecules. The mesoporous catalysts were used as an oxidative nano-reactor in
heterogeneous catalytic reactions to afford highly fluorescent poly(methylene anthracene)s (PMAn) when anthracene
was used as a monomer. The structure of the mesoporous Fe-SBA15 was 2D channel with large surface area of 710 m2/g
and pore size of 9.2 nm. The fluorescent polymer was synthesized with high yield of 90 % in short reaction time. The
synthesized polymer PMAn showed good emission properties with high excimer emission, which was highly affected by
the pore size of the reactor. This indicated that the optical properties of fluorescent polymers synthesized from this
method could be controlled by the pore size of the mesoporous templates.
Jeonghun Kim,Chokkalingam Anand,Jungmok You,Yuna Kim,Byeonggwan Kim,Ajayan Vinu, andEunkyoung Kim
"Template assisted polymerization of functional materials and their
opto-electronic properties", Proc. SPIE 7935, Organic Photonic Materials and Devices XIII, 79350L (21 February 2011); https://doi.org/10.1117/12.874306
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Jeonghun Kim, Chokkalingam Anand, Jungmok You, Yuna Kim, Byeonggwan Kim, Ajayan Vinu, Eunkyoung Kim, "Template assisted polymerization of functional materials and their opto-electronic properties," Proc. SPIE 7935, Organic Photonic Materials and Devices XIII, 79350L (21 February 2011); https://doi.org/10.1117/12.874306