Taxonomy, chemical bonding relations and nonlinear optical properties of noncentrosymmetric sulfide crystals

Laiming Zhang; Victor Atuchin; Boris Kidyarov; Yury Andreev

doi:10.1117/12.2010566

16 May 2013 Taxonomy, chemical bonding relations and nonlinear optical properties of noncentrosymmetric sulfide crystals

Laiming Zhang, Victor Atuchin, Boris Kidyarov, Yury Andreev

Author Affiliations +

Proceedings Volume 8796, 2nd International Symposium on Laser Interaction with Matter (LIMIS 2012); 87962A (2013) https://doi.org/10.1117/12.2010566
Event: 2nd International Symposium on Laser Interaction with Matter (LIMIS 2012), 2012, Xi'an, Shaanxi, China

Abstract

A set of ~450 noncentrosymmetric sulfides has been observed in reference to nonlinear optical properties. It has been found that on the plane of the oxide bond lengths the noncentrosymmetric sulfide crystals are dominantly positioned into a rosette of two intersected ellipses of «acentricity». The strongly non-monotonic dependency of nonlinear optical susceptibility χ⁽²⁾ on the shortest chemical bond length L(E,M-S) has been obtained for sulfides. The suggested crystal chemistry analysis is useful for searching new noncentrosymmetric sulfide crystals.

Citation Download Citation

Laiming Zhang, Victor Atuchin, Boris Kidyarov, and Yury Andreev "Taxonomy, chemical bonding relations and nonlinear optical properties of noncentrosymmetric sulfide crystals", Proc. SPIE 8796, 2nd International Symposium on Laser Interaction with Matter (LIMIS 2012), 87962A (16 May 2013); https://doi.org/10.1117/12.2010566

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