Optical systems modeling and experimental realization of pump and probe technique: investigation of nonlinear absorption in colloidal quantum dots

A. Smirnov; A. Golinskaya; K. Ezhova; M. Kozlova; V. Dneprovskii

doi:10.1117/12.2227855

27 April 2016 Optical systems modeling and experimental realization of pump and probe technique: investigation of nonlinear absorption in colloidal quantum dots

A. Smirnov, A. Golinskaya, K. Ezhova, M. Kozlova, V. Dneprovskii

Author Affiliations +

Proceedings Volume 9889, Optical Modelling and Design IV; 98890R (2016) https://doi.org/10.1117/12.2227855
Event: SPIE Photonics Europe, 2016, Brussels, Belgium

Abstract

Two optical systems modeling of laser and broadband radiation focusing, that is necessary for realization of the pump and probe method, was carried out in this work. Modeling was utilized to construct experimental setup for transmission spectra measuring of studied sample by probe nanosecond broadband radiation (coumarin photoluminescence) depending on the intensity of the nanosecond laser pump pulses. The saturation effect of absorption and the induced charge Stark-effect coexistence and predominate issue of these effects are determined by power of optical excitation. In dependence of tuning of excitation radiation frequency from basic exciton transition frequency nonlinear effects in colloidal CdSe/ZnS quantum dots has been investigated.

Citation Download Citation

A. Smirnov, A. Golinskaya, K. Ezhova, M. Kozlova, and V. Dneprovskii "Optical systems modeling and experimental realization of pump and probe technique: investigation of nonlinear absorption in colloidal quantum dots", Proc. SPIE 9889, Optical Modelling and Design IV, 98890R (27 April 2016); https://doi.org/10.1117/12.2227855

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